著者

Sheng Xu Luyuan Zhang Stewart P. H. T. Freeman Xiaolin Hou Katsuhiko Yamaguchi Alan J. Cresswell David C. W. Sanderson

出版者

GEOCHEMICAL SOCIETY OF JAPAN

雑誌

GEOCHEMICAL JOURNAL (ISSN:00167002)

巻号頁・発行日

vol.50, no.3, pp.287-291, 2016-05-18 (Released:2016-05-30)

参考文献数

18

被引用文献数

3

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This paper reports iodine (127I and 129I) and cesium (137Cs) isotope concentrations in groundwater of confined and unconfined aquifers in the vicinity of the Fukushima Dai-ichi nuclear power plant (FDNPP). 127I and 129I concentrations range from 2–13 μg/L and 5 × 107–8 × 1010 atom/L respectively, resulting in 129I/127I atomic ratios from 5 × 10–9 to 2 × 10–6. In all samples, 137Cs concentrations were below detection limit. The deep-sealed groundwater from the confined aquifer did not contain significant quantities of Fukushima-derived 129I compared to the groundwater in the unconfined aquifer. The minimal 129I/137Cs activity ratios in the groundwater are more than 2–500 times higher than the FDNPP source ratio. These data can be explained by rainwater infiltrating through the surface soils, with the more water-soluble 129I preferentially extracted into the aqueous phase and the 137Cs preferentially retained in the soil.

著者

Mamoru Sato Kaori Matsuoka Tsugiko Takase Natsuko I. Kobayashi Hidetoshi Kikunaga Daisuke Takata Keitaro Tanoi Tsutomu Ohtsuki Shinnosuke Kusaba Katsuhiko Yamaguchi

出版者

The Japanese Society for Horticultural Science

雑誌

The Horticulture Journal (ISSN:21890102)

巻号頁・発行日

pp.UTD-006, (Released:2019-01-18)

被引用文献数

8

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We investigated the vertical 137Cs distribution in soil among five sod culture orchards with different soil textures over six years after 2011, when 137Cs fallout was released by the Fukushima Daiichi Nuclear Power Plant accident, to confirm the long-term 137Cs downward-migration into soil. At each orchard, soil cores were collected to a depth of 30 cm and subdivided into intervals of 3 to 9 cm. The 137Cs within the 3 cm of topsoil decreased from 84–94% during the first 7 months after deposition in 2011 to 41–75% in 2017. From 2012 onward, the vertical 137Cs profiles in the soils were explained by a two-component negative exponential model composed of a rapid and a slow component with a change of slope at a depth of 6 to 9 cm. It took 4 years after deposition to show a significant difference in the value of the average 137Cs migration distance (Md) among the orchards. The speed of 137Cs migration in the orchards during the 6 years after the accident year was 0.44 to 0.97 cm year−1 based on the Md. There was a significant positive correlation between Md and fine sand content in the 3 cm of topsoil between Md and the ratio of the total carbon content (TC) at a depth of 3 to 6 cm to that in the top 3 cm of soil. Furthermore, the percentage of exchangeable 137Cs (ex-137Cs) to 137Cs at 3 to 6 cm depth increased significantly in proportion to the ratio of TC at 3 to 6 cm depth to TC at 0 to 3 cm depth in soil collected in 2013. These findings indicate that one of the mobile forms of 137Cs was ex-137Cs combined with TC and that the fine sand content and TC influenced the 137Cs downward-migration in the 3 cm of topsoil in the orchard in which organic matter accumulated by sod culture.