著者

CHANDRA Naveen PATRA Prabir K. BISHT Jagat S. H. ITO Akihiko UMEZAWA Taku SAIGUSA Nobuko MORIMOTO Shinji AOKI Shuji JANSSENS-MAENHOUT Greet FUJITA Ryo TAKIGAWA Masayuki WATANABE Shingo SAITOH Naoko CANADELL Josep G.

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2021-015, (Released:2020-12-04)

被引用文献数

38

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Methane (CH4) is an important greenhouse gas and plays a significant role in tropospheric and stratospheric chemistry. Despite the relevance of methane (CH4) in human-induced climate change and air pollution chemistry, there is no scientific consensus on the causes of changes in its growth rates and variability over the past three decades. We use a well-validated chemistry-transport model for simulating CH4 concentration and estimation of regional CH4 emissions by inverse modelling for the period of 1988-2016. The control simulations are performed using a seasonally varying hydroxyl (OH) concentrations and assumed no interannual variability. Using inverse modelling of atmospheric observations, emission inventories, a wetland model, and a δ13C-CH4 box model, we show that reductions in emissions from Europe and Russia since 1988, particularly from oil-gas exploitation and enteric fermentation, led to decreased CH4 growth rates in the 1990s. This period was followed by a quasi-stationary state of CH4 in the atmosphere during the early 2000s. CH4 resumed growth from 2007, which we attribute to increases in emissions from coal mining mainly in China and intensification of ruminant farming in tropical regions. A sensitivity simulation using interannually varying OH shows that regional emission estimates by inversion are unaffected for the mid- and high latitude areas. We show that meridional shift in CH4 emissions toward the lower latitudes and the increase in CH4 loss by hydroxyl (OH) over the tropics finely balance out, which keep the CH4 gradients between the southern hemispheric tropical and polar sites relatively unchanged during 1988-2016. The latitudinal emissions shift is confirmed using the global distributions of the total column CH4 observations by satellite remote sensing. There is no evidence of emission enhancement due to climate warming, including the boreal regions, during our analysis period. These findings highlight key sectors for effective emission reduction strategies toward climate change mitigation.

著者

UMEZAWA Taku ANDREWS Stephen J. SAITO Takuya

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2020-007, (Released:2019-11-10)

被引用文献数

1

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Although methane plays an important role in climate change and atmospheric chemistry, its global budget remains quantitatively uncertain due mainly to a wide variety of source types. The stable carbon isotope ratio of atmospheric methane (δ13C-CH4) is useful for separating contributions of different source categories, but due to the complex and laborious analysis, limited measurement data exists. We present a new system for δ13C-CH4 measurement, optimized for the automated analysis of air samples. Although the system is designed in principle similarly to those in previous studies, we successfully set up the system with no use of cryogens (e.g. liquid nitrogen) and attained reproducibility sufficient to analyze atmospheric variations (∼ 0.1 ‰). We performed automated continuous measurements of ambient air outside our laboratory at about hourly intervals for 2 months, which characterized imprint of local methane sources well. Future measurement operation for flask air samples from existing atmospheric monitoring programs will provide a large number of atmospheric δ13C-CH4 data.