著者

ISHIJIMA Kentaro TSUBOI Kazuhiro MATSUEDA Hidekazu TANAKA Taichu Yasumichi MAKI Takashi NAKAMURA Takashi NIWA Yosuke HIRAO Shigekazu

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2022-017, (Released:2021-12-10)

被引用文献数

2

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Temporal variations of atmospheric radon-222 (222Rn) observed at four Japan Meteorological Agency stations in Japan by the Meteorological Research Institute were analyzed using an on-line Global Spectral Atmosphere Model–Transport Model (GSAM-TM). Monthly and diurnal variations, and a series of synoptic high-222Rn events were extracted from 5-12 years of 222Rn observations during 2007-2019. Observed seasonal patterns of winter maxima and summer minima, driven mainly by monsoons, were well reproduced by the GSAM-TM based on existing 222Rn emission inventories, but their absolute values were generally underestimated, indicating that our understanding of 222Rn emission processes in East Asia is lacking. The high-resolution model (∼ 60 km mesh) demonstrated that observed consecutive high-222Rn peaks at several-hour timescales were caused by two 222Rn streams from different regions and were not well resolved by the low-resolution model (∼ 200 km mesh). GSAM-TM simulations indicate that such cold-front-driven events are sometimes accompanied by complicated three-dimensional atmospheric structures such as stratospheric intrusion over the front, significantly affecting distributions of atmospheric components. A new calculation approach using hourly 222Rn values normalized to daily means was used to analyze the diurnal 222Rn cycle, allowing diurnal cycles in winter to be extracted from 222Rn data that are highly variable due to sporadic continental 222Rn outflows, which tend to obscure the diurnal variations. Normalized diurnal cycles of 222Rn in winter are consistent between observations and model simulations, and seem to be driven mainly by diurnal variations of planetary-boundary-layer height (PBLH). These results indicate that 222Rn in the near-surface atmosphere, transported from remote source regions, could vary diurnally by up to 10 % of the daily mean owing mainly to local PBLH variations, even without significant local 222Rn emissions.

著者

TOHJIMA Yasunori NIWA Yosuke TSUBOI Kazuhiro SAITO Kazuyuki

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2022-021, (Released:2021-12-28)

被引用文献数

2

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Synoptic-scale variabilities of atmospheric CO2 and CH4 observed at Yonagunijima (Yonaguni Island, YON, 24.47°N, 123.01°E) during winter (from January to March) in 1998-2020 were examined. The monthly mean variability ratios (ΔCO2/ΔCH4) based on correlation slopes within 24-hour time windows showed a clear increasing trend, which is mainly attributed to the unprecedented increase in the fossil fuel-derived CO2 (FFCO2) emissions from China. A similar increasing trend of the ΔCO2/ΔCH4 ratio had been reported for the observation at Hateruma Island (HAT, 24.06°N, 123.81°E), located at about 100 km east of YON. However, the absolute values for YON were 34 % larger than those for HAT. In addition, the monthly average in February 2020 for YON showed no marked change, while that for HAT showed an abrupt considerable decrease associated with the FFCO2 emission decrease in China presumably caused by the COVID-19 lockdown. Investigating the diurnal variations, we found that the local influences were larger at YON, especially during daytime, than at HAT. Using nighttime data (20-6 LST) and a longer time window (84-hour), we succeeded in reducing the local influences and the resulting monthly mean ΔCO2/ΔCH4 ratio showed considerable similarity to that observed at HAT including the abrupt decrease in February 2020. These results convinced us that the ΔCO2/ΔCH4 ratio could be successfully used to investigate the relative emission strength in the upwind region.