著者

ISHIJIMA Kentaro TSUBOI Kazuhiro MATSUEDA Hidekazu TANAKA Taichu Yasumichi MAKI Takashi NAKAMURA Takashi NIWA Yosuke HIRAO Shigekazu

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2022-017, (Released:2021-12-10)

被引用文献数

2

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Temporal variations of atmospheric radon-222 (222Rn) observed at four Japan Meteorological Agency stations in Japan by the Meteorological Research Institute were analyzed using an on-line Global Spectral Atmosphere Model–Transport Model (GSAM-TM). Monthly and diurnal variations, and a series of synoptic high-222Rn events were extracted from 5-12 years of 222Rn observations during 2007-2019. Observed seasonal patterns of winter maxima and summer minima, driven mainly by monsoons, were well reproduced by the GSAM-TM based on existing 222Rn emission inventories, but their absolute values were generally underestimated, indicating that our understanding of 222Rn emission processes in East Asia is lacking. The high-resolution model (∼ 60 km mesh) demonstrated that observed consecutive high-222Rn peaks at several-hour timescales were caused by two 222Rn streams from different regions and were not well resolved by the low-resolution model (∼ 200 km mesh). GSAM-TM simulations indicate that such cold-front-driven events are sometimes accompanied by complicated three-dimensional atmospheric structures such as stratospheric intrusion over the front, significantly affecting distributions of atmospheric components. A new calculation approach using hourly 222Rn values normalized to daily means was used to analyze the diurnal 222Rn cycle, allowing diurnal cycles in winter to be extracted from 222Rn data that are highly variable due to sporadic continental 222Rn outflows, which tend to obscure the diurnal variations. Normalized diurnal cycles of 222Rn in winter are consistent between observations and model simulations, and seem to be driven mainly by diurnal variations of planetary-boundary-layer height (PBLH). These results indicate that 222Rn in the near-surface atmosphere, transported from remote source regions, could vary diurnally by up to 10 % of the daily mean owing mainly to local PBLH variations, even without significant local 222Rn emissions.

著者

KAJINO Mizuo DEUSHI Makoto SEKIYAMA Tsuyoshi Thomas OSHIMA Naga YUMIMOTO Keiya TANAKA Taichu Yasumichi CHING Joseph HASHIMOTO Akihiro YAMAMOTO Tetsuya IKEGAMI Masaaki KAMADA Akane MIYASHITA Makoto INOMATA Yayoi SHIMA Shin-ichiro TAKAMI Akinori SHIMIZU Atsushi HATAKEYAMA Shiro SADANAGA Yasuhiro IRIE Hitoshi ADACHI Kouji ZAIZEN Yuji IGARASHI Yasuhito UEDA Hiromasa MAKI Takashi MIKAMI Masao

出版者

Meteorological Society of Japan

雑誌

気象集誌. 第2輯 (ISSN:00261165)

巻号頁・発行日

pp.2019-020, (Released:2018-12-09)

被引用文献数

36

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Model performance of a regional-scale meteorology – chemistry model (NHM-Chem) has been evaluated for the consistent predictions of the chemical, physical, and optical properties of aerosols. These properties are essentially important for the accurate assessment of air quality and health hazards, contamination of land and ocean ecosystems, and regional climate changes due to aerosol-cloud-radiation interaction processes. Currently, three optional methods are available: the 5-category non-equilibrium, 3-category non-equilibrium, and bulk equilibrium methods. These three methods are suitable for the predictions of regional climate, air quality, and operational forecasts, respectively. In this paper, the simulated aerosol chemical, physical, and optical properties and their consistency were evaluated by using various observation data in East Asia. The simulated mass, size, and deposition of SO42- and NH4+ agreed well with the observations, whereas those of NO3-, sea-salt, and dust needed improvement. The simulated surface mass concentration (PM10 and PM2.5) and spherical extinction coefficient agreed well with the observations. The simulated aerosol optical thickness and dust extinction coefficient were significantly underestimated.